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Exercises in nonlinear optical spectroscopy - NOOE219
Title: Cvičení z nelineární optické spektroskopie
Guaranteed by: Institute of Physics of Charles University (32-FUUK)
Faculty: Faculty of Mathematics and Physics
Actual: from 2022
Semester: summer
E-Credits: 1
Hours per week, examination: summer s.:0/1, C [HT]
Capacity: unlimited
Min. number of students: unlimited
4EU+: no
Virtual mobility / capacity: no
State of the course: taught
Language: Czech, English
Teaching methods: full-time
Teaching methods: full-time
Guarantor: RNDr. Pavel Malý, Ph.D.
doc. Mgr. Tomáš Mančal, Ph.D.
Annotation -
Last update: prof. RNDr. Marek Procházka, Ph.D. (26.05.2022)
Extension exercises to the lecture Nonlinear Optical Spectroscopy (NOOE119) will introduce students theoretically to concrete implementations and results of contemporary nonlinear spectroscopy methods.
Aim of the course -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

To introduce students theoretically to contemporary implementations of nonlinear spectroscopy methods. To show the manifestation of the properties of the measured systems and their dynamics in the measured spectra using concrete examples and data.

Course completion requirements -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

Calculation of a nonlinear spectroscopy problem selected by the student.
Literature -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

Shaul Mukamel, Principles of nonlinear optical spectroscopy

L. Valkunas, D. Abramavičius and T. Mančal, Molecular Excitation Dynamics and Relaxation: Quantum Theory and Spectroscopy

P. Hamm and M. Zanni, Concepts and Methods of 2D Infrared Spectroscopy

Selected papers

Teaching methods -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

In-person exercise
Requirements to the exam -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

Theoretical knowledge of basic implementations of methods and applications of nonlinear spectroscopy
Syllabus -
Last update: RNDr. Pavel Malý, Ph.D. (25.05.2022)

Excited molecule model as a displaced oscillator with an explicit vibrational mode in a harmonic bath.

Absorption spectrum as a linear response and its relation to the population-detected excitation spectrum. Franck-Condon and Huang-Rhys factors.

(Relationship of coherent dynamics and Pauli governing equations, Einstein coefficients microscopically)

Principles of construction of nonlinear measurements. Phase-matching geometries. Phase-cycling schemes.

Third-order coherent spectroscopy: from pump-probe to 2DES.

Homogeneous and inhomogeneous broadening, energy transfer, vibrational oscillations.

Global analysis of spectra.

Overview of currently developed methods, coherent vs population detection, nonlinearities of other orders.

 
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